Thanks for the tip. I haven't heard at least about 20% of his albums, but I will check out the ones you recommend.
In truth, I recommend Neil Young & Crazy Horse. Studio and live. That's the best stuff (IMO). I love This Notes For You (jazzy blues album with a horn section). The album with Pearl Jam (Mirrorball) is not too bad. His archive stuff from early 70s is excellent too.
Neil Young and Crazy Horse - Ragged Glory is a good one.
That was my favorite for years. Now I lean slightly towards Broken Arrow. I hate Green whatever (the musical) Sleeps With Angels is decent, and Psychedelic Pill is actually quite good, considering their advanced age. 
I might get hate for this, but I love Neil Young's Trans album. It's exactly what I want Kraftwerk to be, not what Kraftwerk actually is
I love Trans and anything like it. I know Homeless_Dad will show up here eventually. It's one of his favorites, too. I was just giving (the) Razor a basic idea where to go next. I'd say Trans is about 5 steps further into the NY wormhole. Have you seen his Berlin live set from the Trans tour? I have the DVD.